1. aimed high- and low-frequency laser beams at a semiconductor
2. electrons were caused to be ripped from their cores, accelerated, and then smashed back into the cores they left behind.
3. This recollision produced multiple frequencies of light simultaneously.
"It's fairly routine to mix the lasers and get one or two new frequencies, Sherwin continued. "But to see all these different new frequencies, up to 11 in our experiment, is the exciting phenomenon. Each frequency corresponds to a different color."
Credit: Peter Allen, UCSB
Nature - Experimental observation of electron–hole recollisions
In terms of real-world applications, the electron-hole recollision phenomenon has the potential to significantly increase the speed of data transfer and communication processes. One possible application involves multiplexing –– the ability to send data down multiple channels –– and another is high-speed modulation.
"Think of your cable Internet," explained Ben Zaks, a UCSB doctoral student in physics and the paper's lead author. "The cable is a bundle of fiber optics, and you're sending a beam with a wavelength that's approximately 1.5 microns down the line. But within that beam there are a lot of frequencies separated by small gaps, like a fine-toothed comb. Information going one way moves on one frequency, and information going another way uses another frequency. You want to have a lot of frequencies available, but not too far from one another."
The electron-hole recollision phenomenon does just that –– it creates light at new frequencies, with optimal separation between them.
The researchers utilize a free electron laser –– a building-size machine in UCSB's Broida Hall –– to produce the electron-hole recollisions, which they note is not practical for real-world applications. Theoretically, however, a transistor could be used in place of the free electron laser to produce the strong terahertz fields. "The transistor would then modulate the near infrared beam," Zaks continued. "Our data indicates that we are modulating the near infrared laser at twice the terahertz frequency. This is where we could really see this working to increase the speed of optical modulation, which is how you get information down a cable line."
The electron-hole recollision phenomenon creates many new avenues for research and exploration, Sherwin noted. "It is an interesting time because there are a lot of people who can participate in doing this kind of research," he said. "We have a unique tool –– a free electron laser –– which gives us a big advantage for exploring the properties of fundamental materials. We just put it in front of our laser beams and measure the colors of light going out. Now that we've seen this phenomenon, we can start doing the hard work of putting the pieces together on a chip."
When the high-frequency optical laser beam hits the semiconductor material –– in this case, gallium arsenide nanostructures –– it creates an electron-hole pair called an exciton. The electron is negatively charged, and the hole is positively charged, and the two are bound together by their mutual attraction. "The high-frequency laser creates electrons and holes," Sherwin explained. "The very strong, low-frequency free electron laser beam rips the electron away from the hole and accelerates it. As the low-frequency field oscillates, it causes the electron to come careening back to the hole." The electron has excess energy because it has been accelerated, and when it slams back into the hole, the recombined electron-hole pair emits photons at new frequencies.
An intense laser field can remove an electron from an atom or molecule and pull the electron into a large-amplitude oscillation in which it repeatedly collides with the charged core it left behind. Such recollisions result in the emission of very energetic photons by means of high-order-harmonic generation, which has been observed in atomic and molecular gases as well as in a bulk crystal. An exciton is an atom-like excitation of a solid in which an electron that is excited from the valence band is bound by the Coulomb interaction to the hole it left behind. It has been predicted that recollisions between electrons and holes in excitons will result in a new phenomenon: high-order-sideband generation. In this process, excitons are created by a weak near-infrared laser of frequency fNIR. An intense laser field at a much lower frequency, fTHz, then removes the electron from the exciton and causes it to recollide with the resulting hole. New emission is predicted to occur as sidebands of frequency fNIR + 2nfTHz, where n is an integer that can be much greater than one. Here we report the observation of high-order-sideband generation in semiconductor quantum wells. Sidebands are observed up to eighteenth order (+18fTHz, or n = 9). The intensity of the high-order sidebands decays only weakly with increasing sideband order, confirming the non-perturbative nature of the effect. Sidebands are strongest for linearly polarized terahertz radiation and vanish when the terahertz radiation is circularly polarized. Beyond their fundamental scientific significance, our results suggest a new mechanism for the ultrafast modulation of light, which has potential applications in terabit-rate optical communications.
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